我组范正龙在Nano Letters上发表论文
Emergent Intrinsic Ferromagnetism in Two-Dimensional Trigonal Rhodium Oxide | |
作者: | Zhenglong Fan,[a]# Yixin Liu,[b]# Xinyuan Wei,[c]# Wenxiang Zhu,[a] Hui Huang,[a] Qi Shao,[a] Fan Liao,[a]Mingwang Shao,[a]* Wei Li,[c]* Gang Mu,[b]* Yang Liu,[a]* and Zhenhui Kang,[a][d]* |
单位: | [a] Institute of Functional Nano and Soft Materials (FUNSOM), Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices, Joint International Research Laboratory of Carbon-Based Functional Materials and Devices, Soochow University, Suzhou 215123, People’s Republic of China. [b]State Key Laboratory of Functional Materials forInformatics, Shanghai Institute of Microsystem andInformation Technology, Chinese Academy of Sciences,Shanghai 200050, China. [c] State Key Laboratory of Surface Physics and Department of Physics, Fudan University, Shanghai 200433,China. [d] Macao Institute of Materials Science and Engineering (MIMSE) MUST-SUDA Joint Research Center for Advanced Functional Materials, Macau University of Science and Technology, Taipa, Macao 999078, China. |
摘要: | Two-dimensional (2D) van der Waals single crystals with long-range magnetic order are the precondition and urgent task for developing a 2D spintronics device. In contrast to graphene and transition metal dichalcogenides, the study of 2D single-crystal metal oxides with intrinsic ferromagnetic properties remains a huge challenge. Here, we report a large-size trigonal single-crystal rhodium oxide (SC-Tri-RhO2), with crystal parameters of a = b = 3.074 Å, c = 6.116 Å, and a space group of P3m1 (164), exhibiting strong ferromagnetism (FM) at a rather high temperature. Furthermore, theoretical calculations suggest that the ferromagnetism in SC-Tri-RhO2 originates from spin splitting near the Fermi level, and the total magnetic moment is contributed mainly by the Rh atom. |
影响因子: | 10.8 |
分区情况: | 1区 |
链接: | https://pubs.acs.org/doi/full/10.1021/acs.nanolett.3c03087 |